A novel variable transformation approach for enhancing conformational sampling in complex systems

Pr. Mark E. Tuckerman, Dept. Of Chemistry and Courant Institute of Mathematical Sciences, New York University, New York, NY 10003
e-mail:???


Mardi 18 juin 2002, 11h00
One of the computational granc challenge problems is to develop methodology capable of sampling conformational equilibria in systems with rough energy landscapes. If met, many important problems, most notably protein folding, could be significantly impacted. In this talk, I will present a new approach in which molecular dunamics is combined with a novel variable transformation designed to wrap configuration space in such a way that barriers are reduced and attractive basins stretched. The new method rigorously preserves equilibrium properties while leading to very large enhancements in sampling effciency. I will also show how the method can be extended to free energy calculations. The performance of the new approach will be demonstrated on simple example problems, long polymer chains, and biologically important systems.