Electronic structure by quantum Monte Carlo methods: molecules, nanoclusters and solids

Lubos Mitas, Raleigh, North-Carolina, U.S.A


Lundi 10 juin 2002, 11h00
Quantum Monte Carlo (QMC) is a modern computational methodology for efficient solving of quantum many-body problems. It is based on a powerful combination of many-body wave functions and robustness of Monte Carlo techniques. The talk will be focused on the electronic structure QMC methods and their applications to real systems. The basic notions of QMC, such as the correlated wave function construction, variational and Green's function Monte Carlo methods will be briefly explained. The QMC applications will include evaluations and predictions of energy ordering of Si and C clusters [1,2,3], cohesive energies and excitations in insulating solids [4,5,6], excitations in molecules [7], barriers in chemical reactions [8], and structures of conjugated carbon rings [9].
The applications will illustrate the main features of QMC: direct and accurate treatment of electron correlation, wide range of applicability, favorable scaling in the number of particles when compared with other correlated methods and scalability on parallel architectures. Perhaps even more important than accurate "numbers" are new insights into the behavior of interacting quantum particles. Recasting of the Schrodinger equation into a stochastic process enables to capture many-particle effects in a very efficient manner and sheds new light on the nature of the correlation problem. The computational efficiency provides opportunities for studies of large systems with hundreds of valence electrons. ie, beyond the reach of traditional correlated wave function approaches. Finally, the current developments and obtained results suggest that QMC has become a powerful predictive tool and a new alternative for accurate electronic structure calculations.
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[9] T. Torelli and L. Mitas, Phys. Rev. Lett. 85, 1702 ('00)