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General considerations

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{\bf Reference literature:...
...newblock {\em J. Chem. Phys.} {\bf 82}, \hspace{0.25em}3235, (1985)
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A response function is a measure of how a property of a system changes in the presence of one or more perturbations. With our notation (see e.g. Ref. [48]), $\langle\!\langle A;B\rangle\!\rangle_{\omega_b}$, $\langle\!\langle A;B,C\rangle\!\rangle_{\omega_b,\omega_c}$, and $\langle\!\langle A;B,C,D\rangle\!\rangle_{\omega_b,\omega_c,\omega_d}$ denote linear, quadratic and cubic response functions, respectively, which provide the first, second, and third-order corrections to the expectation-value of $A$, due to the perturbations $B$, $C$, and $D$, each of which is associated with a frequency $\omega_b$, $\omega_c$, and $\omega_d$. Often the perturbations are considered to be external monochromatic fields, or static (e.g. relativistic) perturbations, in which case the frequency is zero. In general, the perturbations $B$, $C$, and $D$ represent Fourier components of an arbitrary time-dependent perturbation.



Dalton Manual - Release 1.2.1